| 3866 |
680 |
Mn3O4 nanozyme coating accelerates nitrate reduction and decreases N2O emission during photoelectrotrophic denitrification by Thiobacillus denitrificans-CdS |
https://doi.org/10.1021/acs.est.0c02709 |
Metal oxide |
This work successfully constructed a Mn3O4 nanozyme-coated biosemiconductor, Thiobacillus denitrificans-cadmium sulfide (T. denitrificans-CdS@Mn3O4), via a simple, fast, and economic method. After Mn3O4 coating, the ROS were greatly eliminated; the concentrations of hydroxyl radicals, superoxide radicals, and hydrogen peroxide were reduced by 90%, 77.6%, and 26%, respectively, during photoelectrotrophic denitrification (PEDeN). T. denitrificans-CdS@Mn3O4 showed a 28% higher rate of nitrate reduction and 78% lower emission of nitrous oxide (at 68 h) than that of T. |